Not sure is it related to the fragmentation, but I can say that serious 
performance degradation in my NFS/ZFS benchmarks [1] is a result of on-disk ZFS 
data layout.
Read operations on directories (NFS3 readdirplus) are abnormally time consuming 
. That kills the server. After cold restart of the host the performans is still 
on the flour. My conclusion: it's not CPU, not memory, it's ZFS on-disk 
structures.

[1] http://www.opensolaris.org/jive/thread.jspa?threadID=24014
 
 
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