Brother,I had same views and after creating some small projects I directly 
tried to jump over large projects (went for data mining using neural network) 
and FAILED.
I realized small things really matter.
So I suggest just couple of GUI projects are not enough go for more.
start with anything.
here are couple of links I am staring with:
1. http://www.reddit.com/r/beginnerprojects
2. http://www.openbookproject.net/py4fun/

and there are many more you can go for "learnstreet.com"

I am too a Intermediate but I prefer to say Beginner and if you want we can 
make projects together.
I am Currently working on a small chat application.
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