Guy Rutenberg schrieb:

Using \renewenvironment didn't work (LyX still treats it as an eqnarray and adds
an extra &).

Sorry my fault, this is of course not possible because align has 2 columns, 
eqnarray 3 columns.

So the easiest way is to define a keyboard shortcut that inserts an align equation. How to define such a shortcut is explained in the Customization manual. (The next major LyX release has a dilaog where you can define them much more easier.)
For existing formulas, use the menu Edit -> Math -> Change formula type 
(shortcut Alt-m t a).

regards Uwe

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